Visualizing Uniaxial-strain Manipulation of Antiferromagnetic

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Nematic phase: the hole pocket distorts, one elongated electron pocket seen by ARPES. DFT calculation In this paper, to our knowledge, we report the first observation of an insulator–superconductor crossover in the iron-based superconductors by performing systematic angle-resolved photoemission (ARPES) measurements on the single-layer FeSe/SrTiO 3 films at various carrier concentrations. We have revealed the existence of a novel electronic state in an highly unconventional multiband superconductor, FeSe, from the evolution of its electronic structure from the high-temperature tetragonal phase into the electronic nematic phase using angle resolved photoemission spectroscopy (ARPES). Bulk FeSe is an iron-based superconductor that has a maximum Tc of 8K. Surprisingly, the Tc of a single layer of FeSe film grown epitaxially on the SrTiO 3 substrate is enhanced to over 55K.

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The gap function is determined in a full Brillouin zone including all Fermi surfaces and kz-dependence. We find significant anisotropy of the superconducting gap in all momentum directions. While the in-plane anisotropy can be explained by both, nematicity-induced pairing anisotropy and We have performed in-situ angle-resolved photoemission spectroscopy measurements of cesium(Cs)-deposited FeSe thin films on SrTiO 3. We found that Cs deposition enables heavily electron doping into the FeSe layer. In properly doped films, we also revealed the occurrence of superconductivity accompanied by the suppression of electronic nematicity.

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We found that Cs deposition enables heavily electron doping into the FeSe layer. In properly doped films, we also revealed the occurrence of superconductivity accompanied by the suppression of electronic nematicity.

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The application of a mechanical strain is used to promote the volume fraction of one of the orthorhombic domains in the sample, which we estimate to be 80% detwinned. While the full structure of the electron pockets consisting of two crossed ellipses may be observed in the tetragonal phase at temperatures above 90 2015-04-16 · The ARPES results on FeSe single crystals reported so far give a basically consistent picture [32, 67, 68], as exemplified in figure 4.

Here, we report high resolution angle resolved photoemission spectroscopy (ARPES) results which reveal an unexpected and unique characteristic of the 1UC FeSe/STO system: each energy band of the FeSe film is almost exactly replicated at a fixed energy separation. Combining Angle resolved photoelectron spectroscopy (ARPES) and a μ-focused Laser, we have performed scanning ARPES microscopy measurements of the domain population within the nematic phase of FeSe single crystals. We are able to demonstrate a variation of the domain population density on a scale of a few 10 μmwhile constraining the upper limit of This is confirmed by performing ARPES on FeSe single crystals, whereby a 25-meV rigid chemical potential shift is detected across the entire Brillouin zone over the temperature range between 100 K and 300 K. The finding has important implications for any future theoretical models of nematicity and superconductivity in FeSe and related materials. the low temperature Fermi surface of FeSe as experimentally determined by ARPES consists of one ellipti-cal hole pocket and one orthogonally-oriented peanut-shaped electron pocket. Our measurements clarify the long-standing controversies over the interpretation of ARPES measurements of FeSe. INTRODUCTION 2012-07-03 · Direct-ARPES and STM Investigation of FeSe Thin Film Growth by Nd:YAG Laser Sandeep Kumar Chaluvadi, Debashis Mondal, Chiara Bigi, Jun Fujii, Rajdeep Adhikari, Regina Ciancio Phase diagram of FeSe 1 − x S x and the suppression of electronic correlations by S substitution.
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At a very low carrier concentration, the spectral The observation of replica bands in single-unit-cell FeSe on SrTiO3 (STO)(001) by angle-resolved photoemission spectroscopy (ARPES) has led to the conjecture that the coupling between FeSe Phase diagram of FeSe 1 − x S x and the suppression of electronic correlations by S substitution.

Combining molecular beam epitaxy and in situ angle resolved photoemission spectroscopy (ARPES), we study the ultra thin FeSe films on 2 RESULTS HolePockets.
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This work was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division under contract DE-AC02-76SF00515. 2017-10-23 · We report high resolution angle-resolved photo-emission spectroscopy (ARPES) measurements of detwinned FeSe single crystals.


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Visualizing Uniaxial-strain Manipulation of Antiferromagnetic

c,d) Spectra and its second derivative taken at zone corner M, along the cut shown with the white line in (b).

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2017-10-23 · We report high resolution angle-resolved photo-emission spectroscopy (ARPES) measurements of detwinned FeSe single crystals. The application of a mechanical strain is used to promote the volume fraction of one of the orthorhombic domains in the sample, which we estimate to be detwinned. The observation of replica bands in single-unit-cell FeSe on SrTiO3 (STO)(001) by angle-resolved photoemission spectroscopy (ARPES) has led to the conjecture that the coupling between FeSe ARPES: schematic Fermi surfaces of FeSe –3D Tetragonal phase: smaller pockets and band renormalisations. Nematic phase: the hole pocket distorts, one elongated electron pocket seen by ARPES. DFT calculation In this paper, to our knowledge, we report the first observation of an insulator–superconductor crossover in the iron-based superconductors by performing systematic angle-resolved photoemission (ARPES) measurements on the single-layer FeSe/SrTiO 3 films at various carrier concentrations.

[37] found the FSs of the monolayer FeSe film and the multilayer FeSe film were significantly different ( Fig. 12 ). Recent ARPES results show that after FeSe films enter the high-T c phase via surface K dosing, the electron correlation anomalously increases upon further doping, and eventually, an insulating phase emerges . This indicates remarkable complexity and new physics in the “overdoped” region. FeSe is a fascinating superconducting material at the frontier of research in condensed matter physics. Here, we provide an overview of the current understanding of the electronic structure of FeSe, focusing in particular on its low-energy electronic structure as determined from angle-resolved photoemission spectroscopy, quantum oscillations, and magnetotransport measurements of single-crystal in bulk FeSe samples [6]. In this wide temperature range, the system shows a marked electron nematicity in transport [7].